Pressure-induced phase transitions of multiferroic BiFeO<SUB>3</SUB>

ZHANG Xiao-Li; WU Ye; ZHANG Qian; DONG Jun-Cai; WU Xiang; LIU Jing; WU Zi-Yu; CHEN Dong-Liang

doi:10.1088/1674-1137/37/12/128001

Chinese Physics C> 2013, Vol. 37> Issue(12) : 128001 DOI: 10.1088/1674-1137/37/12/128001

Pressure-induced phase transitions of multiferroic BiFeO₃

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Abstract：
Pressure-induced phase transitions of multiferroic BiFeO₃ have been investigated using synchrotron radiation X-ray diffraction with diamond anvil cell technique at room temperature. Present experimental data clearly show that rhombohedral (R3c) phase of BiFeO₃ first transforms to monoclinic (C2/m) phase at 7 GPa, then to orthorhombic (Pnma) phase at 11 GPa, which is consistent with recent theoretical ab initio calculation. However, we observe another peak at 2θ=7° in the pressure range of 5-7 GPa that has not been reported previously. Further analysis reveals that this reflection peak is attributed to the orthorhombic (Pbam) phase, indicating the coexistance of monoclinic phase with orthorhombic phase in low pressure range.

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ZHANG Xiao-Li, WU Ye, ZHANG Qian, DONG Jun-Cai, WU Xiang, LIU Jing, WU Zi-Yu and CHEN Dong-Liang. Pressure-induced phase transitions of multiferroic BiFeO₃[J]. Chinese Physics C, 2013, 37(12): 128001. doi: 10.1088/1674-1137/37/12/128001

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Received: 2013-03-13
Revised: 2013-07-02

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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Pressure-induced phase transitions of multiferroic BiFeO₃

Corresponding author: WU Xiang,

Corresponding author: WU Zi-Yu,

Corresponding author: CHEN Dong-Liang,

Received Date: 2013-03-13

Accepted Date: 2013-07-02

Available Online: 2013-12-05

Abstract: Pressure-induced phase transitions of multiferroic BiFeO₃ have been investigated using synchrotron radiation X-ray diffraction with diamond anvil cell technique at room temperature. Present experimental data clearly show that rhombohedral (R3c) phase of BiFeO₃ first transforms to monoclinic (C2/m) phase at 7 GPa, then to orthorhombic (Pnma) phase at 11 GPa, which is consistent with recent theoretical ab initio calculation. However, we observe another peak at 2θ=7° in the pressure range of 5-7 GPa that has not been reported previously. Further analysis reveals that this reflection peak is attributed to the orthorhombic (Pbam) phase, indicating the coexistance of monoclinic phase with orthorhombic phase in low pressure range.

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Pressure-induced phase transitions of multiferroic BiFeO₃

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Pressure-induced phase transitions of multiferroic BiFeO₃

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Pressure-induced phase transitions of multiferroic BiFeO3

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通讯作者: 陈斌, bchen63@163.com

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Pressure-induced phase transitions of multiferroic BiFeO3

Corresponding author: WU Xiang,

Corresponding author: WU Zi-Yu,

Corresponding author: CHEN Dong-Liang,

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Pressure-induced phase transitions of multiferroic BiFeO₃

Pressure-induced phase transitions of multiferroic BiFeO₃